Publications by Type: Journal Article

2017
Chenghe Guan and Peter Rowe. 2017. “In pursuit of a well-balanced network of cities and towns: A case study of the Changjiang Delta Region.” Environment and Planning B: Urban Analytics and City Science, 48, 3, Pp. 1-19. Publisher's VersionAbstract
Development of urban networks of cities and towns has received attention including discussions of tensions between population concentrations and overlaps with environmentally sensitive and disaster-prone areas. Moreover, certain development in broad regions of China, such as its deltas, has become a subject of debate. Contrary to some assumptions, this development within places like the Changjiang Delta (also known as the Yangtze River Delta) has proceeded in a relatively incremental manner. However, at this juncture, controlled development of larger cities, like Shanghai, has shifted to more conventional urbanization pathways forward involving larger city expansions. Nevertheless, further urban growth management appears to depend on development and maintenance of a well-balanced network of large, medium, and small-scaled cities and towns. An important aspect of this development involves definition of the Changjiang Delta region itself, and in particular, alongside its likely further economic performance. To these ends, a scenario-based Cellular Automata model of spatial distribution is deployed, reflecting separate thematic projections. A baseline for economic performance is developed, incorporating measures of fixed-asset investment in urban service, revenue from urban maintenance, and Gross Domestic Product. Revelation of a well-performing network involves spatial distribution of development at various scales, and in various concentrations within the region, moreover, location of this development, largely perpendicular to well-travelled corridors, appears as a preferable outcome, contrary to earlier depictions along the major transportation corridors.
Xinyu Chen, Michael B. McElroy, and Chongqing Kang. 2017. “Integrated energy systems for higher wind penetration in China: Formulation, implementation, and impacts.” IEEE Transactions on Power Systems, 33, 2, Pp. 1309-1319. Publisher's VersionAbstract
With the largest installed capacity in the world, wind power in China is experiencing a ∼20% curtailment. The inflexible combined heat and power (CHP) has been recognized as the major barrier for integrating the wind source. The approach to reconcile the conflict between inflexible CHP units and variable wind power in Chinese energy system is yet un-clear. This paper explores the technical and economic feasibility of deploying the heat storage tanks and electric boilers under typical power grids and practical operational regulations. A mixed integer linear optimization model is proposed to simulate an integrated power and heating energy systems, including a CHP model capable of accounting for the commitment decisions and non-convex energy generation constraints. The model is applied to simulate a regional energy system (Jing-Jin-Tang) covering 100-million population, with hourly resolution over a year, incorporating actual data and operational regulations. The results project an accelerating increase in wind curtailment rate at elevated wind penetration. Investment for wind breaks-even at 14% wind penetration. At such penetration, the electric boiler (with heat storage) is effective in reducing wind curtailment. The investment in electric boilers is justified on a social economic basis, but the revenues for different stakeholders are not distributed evenly.
Haikun Wang, Yanxu Zhang, Xi Lu, Weimo Zhu, Chris P. Nielsen, Jun Bi, and Michael B. McElroy. 2017. “Trade‐driven relocation of air pollution and health impacts in China.” Nature Communications, 8, 738. Publisher's VersionAbstract
Recent studies show that international trade affects global distributions of air pollution andpublic health. Domestic interprovincial trade has similar effects within countries, but has notbeen comprehensively investigated previously. Here we link four models to evaluate theeffects of both international exports and interprovincial trade on PM2.5pollution and publichealth across China. We show that 50–60% of China’s air pollutant emissions in 2007 wereassociated with goods and services consumed outside of the provinces where they wereproduced. Of an estimated 1.10 million premature deaths caused by PM2.5pollutionthroughout China, nearly 19% (208,500 deaths) are attributable to international exports. Incontrast, interprovincial trade leads to improved air quality in developed coastal provinceswith a net effect of 78,500 avoided deaths nationwide. However, both international exportand interprovincial trade exacerbate the health burdens of air pollution in China’s lessdeveloped interior provinces. Our results reveal trade to be a critical but largely overlookedconsideration in effective regional air quality planning for China.
Nan Zhong, Jing Cao, and Yuzhu Wang. 2017. “Traffic congestion, ambient air pollution and health: Evidence from driving restrictions in Beijing.” Journal of the Association of Environmental and Resource Economists, 4, 3, Pp. 821–856. Publisher's VersionAbstract

Vehicles have recently overtaken coal to become the largest source of air pollution in urban China. Research on mobile sources of pollution has foundered due both to inaccessibility of Chinese data on health outcomes and strong identifying assumptions. To address these, we collect daily ambulance call data from the Beijing Emergency Medical Center and combine them with an idiosyncratic feature of a driving restriction policy in Beijing that references the last digit of vehicles’ license plate numbers. Because the number 4 is considered unlucky by many in China, it tends to be avoided on license plates. As a result, days on which the policy restricts license plates ending in 4 unintentionally allow more vehicles in Beijing. Leveraging this variation, we find that traffic congestion is indeed 22% higher on days banning 4 and that 24-hour average concentration of NO2 is 12% higher. Correspondingly, these short term increases in pollution increase ambulance calls by 12% and 3% for fever and heart related symptoms, while no effects are found for injuries. These findings suggest that traffic congestion has substantial health externalities in China but that they are also responsive to policy. 

Michael B. McElroy and Xinyu Chen. 2017. “Wind and solar power in the United States: Status and prospects.” CSEE Journal of Power and Energy Systems, 3, 1. Publisher's VersionAbstract

 

The United States has committed to reduce its greenhouse gas emissions by 26%–28% by 2025 and by 83% by 2050 relative to 2005. Meeting these objectives will require major investments in renewable energy options, particularly wind and solar. These investments are promoted at the federal level by a variety of tax credits, and at the state level by requirements for utilities to include specific fractions of renewable energy in their portfolios (Renewable Portfolio Standards) and by opportunities for rooftop PV systems to transfer excess power to utilities through net metering, allowing meters to operate in reverse. The paper discusses the current status of these incentives.

 

Peter Sherman, Xinyu Chen, and Michael B. McElroy. 2017. “Wind-generated electricity in China: Decreasing potential, inter-annual variability, and association with climate change.” Scientific Reports, 7. Publisher's VersionAbstract
China hosts the world’s largest market for wind-generated electricity. The financial return and carbon reduction benefits from wind power are sensitive to changing wind resources. Wind data derived from an assimilated meteorological database are used here to estimate what the wind generated electricity in China would have been on an hourly basis over the period 1979 to 2015 at a geographical resolution of approximately 50 km × 50 km. The analysis indicates a secular decrease in generating potential over this interval, with the largest declines observed for western Inner Mongolia (15 ± 7%) and the northern part of Gansu (17 ± 8%), two leading wind investment areas. The decrease is associated with long-term warming in the vicinity of the Siberian High (SH), correlated also with the observed secular increase in global average surface temperatures. The long-term trend is modulated by variability relating to the Pacific Decadal Oscillation (PDO) and the Arctic Oscillation (AO). A linear regression model incorporating indices for the PDO and AO, as well as the declining trend, can account for the interannual variability of wind power, suggesting that advances in long-term forecasting could be exploited to markedly improve management of future energy systems.
Science_Reports_Full_Text
2016
Yinmin Xia, Yu Zhao, and Chris P. Nielsen. 2016. “Benefits of China's efforts in gaseous pollutant control indicated by bottom-up emissions and satellite observations 2000-2014.” Atmospheric Environment, 136, July, Pp. 43-53. Publisher's VersionAbstract

To evaluate the effectiveness of national air pollution control policies, the emissions of SO2, NOX, CO and CO2 in China are estimated using bottom-up methods for the most recent 15-year period (2000–2014). Vertical column densities (VCDs) from satellite observations are used to test the temporal and spatial patterns of emissions and to explore the ambient levels of gaseous pollutants across the country. The inter-annual trends in emissions and VCDs match well except for SO2. Such comparison is improved with an optimistic assumption in emission estimation that the emission standards for given industrial sources issued after 2010 have been fully enforced. Underestimation of emission abatement and enhanced atmospheric oxidization likely contribute to the discrepancy between SO2 emissions and VCDs. As suggested by VCDs and emissions estimated under the assumption of full implementation of emission standards, the control of SO2 in the 12th Five-Year Plan period (12th FYP, 2011–2015) is estimated to be more effective than that in the 11th FYP period (2006–2010), attributed to improved use of flue gas desulfurization in the power sector and implementation of new emission standards in key industrial sources. The opposite was true for CO, as energy efficiency improved more significantly from 2005 to 2010 due to closures of small industrial plants. Iron & steel production is estimated to have had particularly strong influence on temporal and spatial patterns of CO. In contrast to fast growth before 2011 driven by increased coal consumption and limited controls, NOX emissions decreased from 2011 to 2014 due to the penetration of selective catalytic/non-catalytic reduction systems in the power sector. This led to reduced NO2 VCDs, particularly in relatively highly polluted areas such as the eastern China and Pearl River Delta regions. In developed areas, transportation is playing an increasingly important role in air pollution, as suggested by the increased ratio of NO2 to SO2 VCDs. For air quality in mega cities, the inter-annual trends in emissions and VCDs indicate that surrounding areas are more influential in NO2 level for Beijing than those for Shanghai.

Challenges faced by China compared with the US in developing wind power
Xi Lu, Michael B. McElroy, Wei Peng, Shiyang Liu, Chris P. Nielsen, and Haikun Wang. 2016. “Challenges faced by China compared with the US in developing wind power.” Nature Energy, 1, 6. Publisher's VersionAbstract

In the 21st Conference of the Parties to the UNFCCC held in Paris in December 2015, China pledged to peak its carbon emissions and increase non-fossil energy to 20% by 2030 or earlier. Expanding renewable capacity, especially wind power, is a central strategy to achieve these climate goals. Despite greater capacity for wind installation in China compared to the US (145.1 versus 75.0 GW), less wind electricity is generated in China (186.3 versus 190.9 TWh). Here, we quantify the relative importance of the key factors accounting for the unsatisfactory performance of Chinese wind farms. Different from the results in earlier qualitative studies, we find that the difference in wind resources explains only a small fraction of the present China-US difference in wind power output (17.9% in 2012); the curtailment of wind power, differences in turbine quality, and delayed connection to the grid are identified as the three primary factors (respectively 49.3%, 50.2%, and 50.3% in 2012). Improvements in both technology choices and the policy environment are critical in addressing these challenges. 

Final Manuscript in DASH
Lu et al. is the cover article of this issue of Nature Energy. It is also subject of a "News and Views" commentary in the same issue, by Joanna I. Lewis.

Qing Yang, Yingquan Chen, Haiping Yang, and Hanping Chen. 2016. “Greenhouse gas emissions of a biomass-based pyrolysis plant in China.” Renewable and Sustainable Energy Reviews, 53, January, Pp. 1580-1590. Publisher's VersionAbstract

Biomass pyrolysis offers an alternative to industrial coal-fired boilers and utilizes low temperature and long residence time to produce syngas, bio-oil and biochar. Construction of biomass-based pyrolysis plants has recently been on the rise in rural China necessitating research into the greenhouse gas emission levels produced as a result. Greenhouse gas emission intensity of a typical biomass fixed-bed pyrolysis plant in China is calculated as 1.55E−02 kg CO2-eq/MJ. Carbon cycle of the whole process was investigated and found that if 41.02% of the biochar returns to the field, net greenhouse gas emission is zero indicating the whole carbon cycle may be renewable. A biomass pyrolysis scenario analysis was also conducted to assess exhaust production, transportation distance and the electricity-generation structure for background information applied in the formulation of national policy.

Jing Cao, Mun S. Ho, and Huifang Liang. 2016. “Household energy demand in urban China: Accounting for regional prices and rapid economic change.” The Energy Journal, 37. Publisher's VersionAbstract

Understanding the rapidly rising demand for energy in China is essential to efforts to reduce the country's energy use and environmental damage. In response to rising incomes and changing prices and demographics, household use of various fuels, electricity and gasoline has changed dramatically in China. In this paper, we estimate both income and price elasticities for various energy types using Chinese urban household micro-data collected by National bureau of Statistics, by applying a two-stage budgeting AIDS model. We find that total energy is price and income inelastic for all income groups after accounting for demographic and regional effects. Our estimated electricity price elasticity ranges from - 0.49 to -0.57, gas price elasticity ranges from -0.46 to -0.94, and gasoline price elasticity ranges from -0.85 to -0.94. Income elasticity for various energy types range from 0.57 to 0.94. Demand for coal is most price and income elastic among the poor, whereas gasoline demand is elastic for the rich.

Rong Xie, Clive E. Sabel, Xi Lu, Weimo Zhu, Haidong Kan, Chris P. Nielsen, and Haikun Wang. 2016. “Long-term trend and spatial pattern of PM2.5-induced premature mortality in China.” Environment International, 97, Pp. 180-186. Publisher's VersionAbstract

With rapid economic growth, China has witnessed increasingly frequent and severe haze and smog episodes over the past decade, posing serious health impacts to the Chinese population, especially those in densely populated city clusters. Quantification of the spatial and temporal variation of health impacts attributable to ambient fine particulate matter (PM2.5) has important implications for China's policies on air pollution control. In this study, we evaluated the spatial distribution of premature deaths in China between 2000 and 2010 attributable to ambient PM2.5 in accord with the Global Burden of Disease based on a high resolution population density map of China, satellite retrieved PM2.5 concentrations, and provincial health data. Our results suggest that China's anthropogenic ambient PM2.5 led to 1,255,400 premature deaths in 2010, 42% higher than the level in 2000. Besides increased PM2.5 concentration, rapid urbanization has attracted large population migration into the more developed eastern coastal urban areas, intensifying the overall health impact. In addition, our analysis implies that health burdens were exacerbated in some developing inner provinces with high population density (e.g. Henan, Anhui, Sichuan) because of the relocation of more polluting and resource-intensive industries into these regions. In order to avoid such national level environmental inequities, China's regulations on PM2.5 should not be loosened in inner provinces. Furthermore policies should create incentive mechanisms that can promote transfer of advanced production and emissions control technologies from the coastal regions to the interior regions.

X.D. Wu, Q. Yang, G.Q. Chen, T. Hayat, and A. Alsaedi. 2016. “Progress and prospect of CCS in China: Using learning curve to assess the cost-viability of a 2x600 MW retrofitted oxyfuel power plant as a case study.” Renewable and Sustainable Energy Reviews, 60, Pp. 1274-1285. Publisher's Version
Meiyu Guo, Xi Lu, Chris P. Nielsen, Michael B. McElroy, Wenrui Shi, Yuntian Chen, and Xuan Yu. 2016. “Prospects for shale gas production in China: Implications for water demand.” Renewable and Sustainable Energy Reviews, 66, December, Pp. 742-750. Publisher's VersionAbstract

Development of shale gas resources is expected to play an important role in China's projected transition to a low-carbon energy future. The question arises whether the availability of water could limit this development. The paper considers a range of scenarios to define the demand for water needed to accommodate China's projected shale gas production through 2020. Based on data from the gas field at Fuling, the first large-scale shale gas field in China, it is concluded that the water intensity for shale gas development in China (water demand per unit lateral length) is likely to exceed that in the US by about 50%. Fuling field would require a total of 39.9–132.9 Mm3 of water to achieve full development of its shale gas, with well spacing assumed to vary between 300 and 1000 m. To achieve the 2020 production goal set by Sinopec, the key Chinese developer, water consumption is projected to peak at 7.22 Mm3 in 2018. Maximum water consumption would account for 1% and 3%, respectively, of the available water resource and annual water use in the Fuling district. To achieve China's nationwide shale gas production goal set for 2020, water consumption is projected to peak at 15.03 Mm3 in 2019 in a high-use scenario. It is concluded that supplies of water are adequate to meet demand in Fuling and most projected shale plays in China, with the exception of localized regions in the Tarim and Jungger Basins.

Ning Zhang, Xi Lu, Chris P Nielsen, Michael B. McElroy, Xinyu Chen, Yu Deng, and Chongqing Kang. 2016. “Reducing curtailment of wind electricity in China by employing electric boilers for heat and pumped hydro for energy storage.” Applied Energy, 184, Pp. 987-994. Publisher's VersionAbstract

Accommodating variable wind power poses a critical challenge for electric power systems that are heavily dependent on combined heat and power (CHP) plants, as is the case for north China. An improved unit-commitment model is applied to evaluate potential benefits from pumped hydro storage (PHS) and electric boilers (EBs) in West Inner Mongolia (WIM), where CHP capacity is projected to increase to 33.8 GW by 2020. A business-as-usual (BAU) reference case assumes deployment of 20 GW of wind capacity. Compared to BAU, expanding wind capacity to 40 GW would allow for a reduction in CO2 emissions of 33.9 million tons, but at a relatively high cost of US$25.3/ton, reflecting primarily high associated curtailment of wind electricity (20.4%). A number of scenarios adding PHS and/or EBs combined with higher levels of wind capacity are evaluated. The best case indicates that a combination of PHS (3.6 GW) and EBs (6.2 GW) together with 40 GW of wind capacity would reduce CO2 emissions by 43.5 million tons compared to BAU, and at a lower cost of US$16.0/ton. Achieving this outcome will require a price-incentive policy designed to ensure the profitability of both PHS and EB facilities.

Yanyang Mei, Qingfeng Che, Qing Yang, Christopher Draper, Haiping Yang, Shihong Zhang, and Hanping Chen. 2016. “Torrefaction of different parts from a corn stalk and its effect on the characterization of products.” Industrial Crops and Products, 92, 15 December, Pp. 26-33. Publisher's VersionAbstract

Torrefaction of biomass can reduce its undesirable properties for the subsequent thermochemical application. After separating a Chinese corn stalk into four parts (leaf, stem, root, and cob), torrefaction was performed at temperatures of 200, 250, and 300 °C respectively. The structural and components differences of various parts were analyzed, along with the solid, gas, and liquid products. The study showed that the root was the most sensitive to heat and the cob showed the biggest increase in CO2 and CO yields with the increase temperature, due to their different content of hemicellulose and cellulose. The torrefaction temperature of 250 °C was especially significant for the formation of acids. Liquid product from the leaf was simpler in composition and lower in yield due to higher content of organic extractives and ash. Generally, various parts have different torrefaction properties due to the differences in chemical composition and cellular structure. And with the thermochemical application of biomass were more widely used in the chemical industry especially fine chemical industry, screening and classification may be necessary.

Yu Deng and Sumeeta Srinivasan. 2016. “Urban land use change and regional access: A case study in Beijing, China.” Habitat International, 51, February, Pp. 103-113. Publisher's VersionAbstract

In the recent past Beijing has experienced rapid development. This growth has been accompanied by many problems including traffic congestion and air pollution. Understanding what stimulates urban growth is important for sustainable development in the coming years. In this paper, we first estimate a binary auto-logistic model of land use change, using physical and socioeconomic characteristics of the location and its access to major centers within the city as predictors. We find that variables determining regional access, like time distance to the city center, the Central Business District (CBD), industrial centers, employment centers, and the transportation system, significantly impact urban land conversion. By using measures of access to predict land use change we believe that we can better understand the planning implications of urban growth not only in Beijing but other rapidly developing cities.

2015
Junling Huang and Michael B. McElroy. 2015. “A 32-year perspective on the origin of wind energy in a warming climate.” Renewable Energy, 77, May, Pp. 482-492. Publisher's VersionAbstract

Based on assimilated meteorological data for the period January 1979 to December 2010, the origin of wind energy is investigated from both mechanical and thermodynamic perspectives, with special focus on the spatial distribution of sources, historical long term variations and the efficiency for kinetic energy production. The dry air component of the atmosphere acts as a thermal engine, absorbing heat at higher temperatures, approximately 256 K, releasing heat at lower temperatures, approximately 252 K. The process is responsible for production of wind kinetic energy at a rate of 2.46 W/m2  sustaining thus the circulation of the atmosphere against frictional dissipation. The results indicate an upward trend in kinetic energy production over the past 32 years, indicating that wind energy resources may be varying in the current warming climate. This analysis provides an analytical framework that can be adopted for future studies addressing the ultimate wind energy potential and the possible perturbations to the atmospheric circulation that could arise as a result of significant exploitation of wind energy.    

Y. Zhao, LP Qiu, RY Xu, FJ Xie, Q. Zhang, YY Yu, C.P. Nielsen, HX Qin, H.K. Wang, XC Wu, WQ Li, and J. Zhang. 2015. “Advantages of city-scale emission inventory for urban air quality research and policy: the case of Nanjing, a typical industrial city in the Yangtze River Delta, China.” Atmospheric Chemistry and Physics, 15, Pp. 12623-12644. Publisher's VersionAbstract

With most eastern Chinese cities facing major air quality challenges, there is a strong need for city-scale emission inventories for use in both chemical transport modeling and the development of pollution control policies. In this paper, a high-resolution emission inventory of air pollutants and CO2 for Nanjing, a typical large city in the Yangtze River Delta, is developed incorporating the best available information on local sources. Emission factors and activity data at the unit or facility level are collected and compiled using a thorough onsite survey of major sources. Over 900 individual plants, which account for 97% of the city's total coal consumption, are identified as point sources, and all of the emission-related parameters including combustion technology, fuel quality, and removal efficiency of air pollution control devices (APCD) are analyzed. New data-collection approaches including continuous emission monitoring systems and real-time monitoring of traffic flows are employed to improve spatiotemporal distribution of emissions. Despite fast growth of energy consumption between 2010 and 2012, relatively small inter-annual changes in emissions are found for most air pollutants during this period, attributed mainly to benefits of growing APCD deployment and the comparatively strong and improving regulatory oversight of the large point sources that dominate the levels and spatial distributions of Nanjing emissions overall. The improvement of this city-level emission inventory is indicated by comparisons with observations and other inventories at larger spatial scale. Relatively good spatial correlations are found for SO2, NOX, and CO between the city-scale emission estimates and concentrations at 9 state-opertated monitoring sites (R = 0.58, 0.46, and 0.61, respectively). The emission ratios of specific pollutants including BC to CO, OC to EC, and CO2 to CO compare well to top-down constraints from ground observations. The inter-annual variability and spatial distribution of NOX emissions are consistent with NO2 vertical column density measured by the Ozone Monitoring Instrument (OMI). In particular, the Nanjing city-scale emission inventory correlates better with satellite observations than the downscaled Multi-resolution Emission Inventory for China (MEIC) does when emissions from power plants are excluded. This indicates improvement in emission estimation for sectors other than power generation, notably industry and transportation. High-resolution emission inventory may also provide a basis to consider the quality of instrumental observations. To further improve emission estimation and evaluation, more measurements of both emission factors and ambient levels of given pollutants are suggested; the uncertainties of emission inventories at city scale should also be fully quantified and compared with those at national scale. 


Yanxia Zhang, Haikun Wang, Sai Liang, Ming Xu, Qiang Zhang, Hongyan Zhao, and Jun Bi. 2015. “A dual strategy for controlling energy consumption and air pollution in China's metropolis of Beijing.” Energy, 81, 1 March, Pp. 294-303. Publisher's VersionAbstract

It is critical to alleviate problems of energy and air pollutant emissions in a metropolis because these areas serve as economic engines and have large and dense populations. Drivers of fossil fuel use and air pollutants emissions were analyzed in the metropolis of Beijing during 1997-2010. The analyses were conducted from both a bottom-up and a top-down perspective based on the sectoral inventories and structural decomposition analysis (SDA). From a bottom-up perspective, the key energy-intensive industrial sectors directly caused the variations in Beijing's air pollution by means of a series of energy and economic policies. From a top-down perspective, variations in production structures caused increases in most materials during 2000-2010, but there were decreases in PM10 and PM2.5 emissions during 2005-2010. Population growth was found to be the largest driver of energy consumption and air pollutant emissions during 1997-2010. This finding suggests that avoiding rapid population growth in Beijing could simultaneously control energy consumption and air pollutant emissions. Mitigation policies should consider not only the key industrial sectors but also socioeconomic drivers to co-reduce energy consumption and air pollution in China's metropolis.

Yu Zhao, Hui Zhong, Jie Zhang, and Chris P Nielsen. 2015. “Evaluating the effects of China's pollution control on inter-annual trends and uncertainties of atmospheric mercury emissions.” Atmospheric Chemistry and Physics, 15, Pp. 4317–4337. Publisher's VersionAbstract
China's atmospheric mercury (Hg) emissions of anthropogenic origin have been effectively restrained through the national policy of air pollution control. Improved methods based on available field measurements are developed to quantify the benefits of Hg abatement through various emission control measures. Those measures include increased use of flue gas desulfurization (FGD) and selective catalyst reduction (SCR) systems for power sector, precalciners with fabric filter (FF) for cement production, machinery coking with electrostatic precipitator (ESP) for iron and steel production, and advanced manufacturing technologies for nonferrous metal smelting. Declining trends in emissions factors for those sources are revealed, leading to a much slower growth of national total Hg emissions than that of energy and economy, from 679 in 2005 to 750 metric tons (t) in 2012. In particular, nearly half of emissions from the above-mentioned four types of sources are expected to be reduced in 2012, attributed to expansion of technologies with high energy efficiencies and air pollutant removal rates after 2005. The speciation of Hg emissions keeps stable for recent years, with the mass fractions of around 55, 39 and 6% for Hg0, Hg2+ and Hgp, respectively. The lower estimate of Hg emissions than previous inventories is supported by limited chemistry simulation work, but middle-to-long term observation on ambient Hg levels is further needed to justify the inter-annual trends of estimated Hg emissions. With improved implementation of emission controls and energy saving, 23% reduction in annual Hg emissions for the most optimistic case in 2030 is expected compared to 2012, with total emissions below 600 t. While Hg emissions are evaluated to be gradually constrained, increased uncertainties are quantified with Monte-Carlo simulation for recent years, particularly for power and certain industrial sources. The uncertainty of Hg emissions from coal-fired power plants, as an example, increased from −48 ~ +73% in 2005 to −50 ~ +89% in 2012 (expressed as 95% confidence interval). This is attributed mainly to swiftly increased penetration of advanced manufacturing and pollutant control technologies. The unclear operation status or relatively small sample size of field measurements on those technologies results in lower but highly varied emission factors. To further confirm the benefits of pollution control polices with reduced uncertainty, therefore, systematic investigations are recommended specific for Hg pollution sources, and the variability of temporal trends and spatial distributions of Hg emissions need to be better tracked for the country under dramatic changes in economy, energy and air pollution status.

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